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Single-photon And Photon-pair Emission From CdSe/Zn(S, Se) Quantum Dots
Published 2003 · Chemistry
We report on the generation of triggered single photons and photon pairs relying on pulsed optical excitation of epitaxially grown self-assembled CdSe quantum dots (QDs). Single-photon emission is studied on individual CdSe/Zn(S,Se) QDs for temperatures up to 200 K. At low temperatures nearly perfect single-photon emission is achieved whereas at higher temperatures an increasing multi-photon emission probability due to spectrally overlapping acoustic phonon sidebands of neighboring QDs is observed. The multi-photon emission probability of a bare QD (background subtracted) is strongly suppressed. Furthermore, the polarization cross correlation of the biexciton-exciton cascade has been investigated in a CdSe/ZnSe QD at low temperatures. A strong polarization correlation of the emitted photon pairs of ∼74% is observed in a linear detection basis.