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High-performance Aqueous Sodium-ion Batteries With K0.27MnO2 Cathode And Their Sodium Storage Mechanism

Y. Liu, Yun Qiao, Wuxing Zhang, Henghui Xu, Zhen Li, Yue Shen, Lixia Yuan, Xianluo Hu, Dai Xiang, Yunhui Huang
Published 2014 · Materials Science

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Abstract Hierarchical layered K 0.27 MnO 2 microflowers are firstly synthesized via a facile and efficient route based on a topochemical reaction process. As cathode materials for aqueous sodium-ion battery, such microflowers exhibit high reversible capacity, long cyclic life and excellent rate capability. After 100 cycles, a reversible capacity of 68.5 mA h g –1 at a current density of 0.2 A g –1 is attained in a full cell with K 0.27 MnO 2 as cathode and NaTi 2 (PO 4 ) 3  as anode. We propose a sodium storage mechanism in K 0.27 MnO 2 by analyzing the evolution of structure and interface during charge/discharge process.
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