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Direct Access To Multi-functionalized Benzenes Via [4 + 2] Annulation Of α-cyano-β-methylenones And α,β-unsaturated Aldehydes

Qianfa Jia, Yunfei Lan, Xin Ye, Yinhe Lin, Qiao Ren

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An efficient [4 + 2] benzannulation of α-cyano-β-methylenones and α,β-unsaturated aldehydes was achieved under metal-free reaction conditions selectively delivering a wide range of polyfunctional benzenes in high yields respectively (up to 94% yield).