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Recent Developments In The Use Of Metal Oxides For Photocatalytic Degradation Of Pharmaceutical Pollutants In Water—a Review

T. Velempini, E. Prabakaran, K. Pillay
Published 2021 · Environmental Science

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Abstract In recent years, metal oxide semiconductors have been explored as photocatalysts for the degradation of organic contaminants in water/wastewater. The uniqueness of these oxide materials is in their ability to harness energy in the UV/Vis range, their relative ease of synthesis, low cost, and their general high surface ratio to mass, etc. Thus, these materials have consequently drawn much profound interest in environment applications, particularly pharmaceutical drugs for photocatalytic degradation. Furthermore, the non-toxic nature of most metal oxide semiconductors means they are convenient for water treatment works, resulting in safe drinking water for humans and safe environments for aquatic mammals. Pharmaceuticals are emerging pollutants that are increasingly being found in water systems. They have been detrimental to the human and animal health. In this article, pharmaceutical drugs abatement from water via photocatalysis process using oxide-based advanced metals such as TiO2, ZnO, Fe2O3,WO3, and Bi2WO6 is discussed. Degradation of various drugs at laboratory scale have been assessed and examples cited. Various approaches to metal oxides modifications and synthesis methods to improve degradation efficiency have also been discussed. Effects of experimental/operational parameters in the degradation process have been compiled and compared. Finally, a short preview of degradation of pharmaceuticals pilot scales is also highlighted.
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A one-step deep eutectic solvent assisted synthesis of carbon nitride/metal oxide composites for photocatalytic nitrogen fixation
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10.1016/J.CEJ.2019.05.041
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10.1016/J.JPHOTOCHEM.2019.111993
Photocatalytic activity of ZnO-WO3 for diclofenac degradation under visible light irradiation
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TiO2 photocatalysis under natural solar radiation for the degradation of the carbapenem antibiotics imipenem and meropenem in aqueous solutions at pilot plant scale.
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Novel Magnetic Carbon Nanotube-TiO2 Composites for Solar Light Photocatalytic Degradation of Pharmaceuticals in the Presence of Natural Organic Matter
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Facile microemulsion synthesis of mesoporous ZnMn2O4 submicrocubes as high-rate and long-life anodes for lithium ion batteries
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10.1016/j.chemosphere.2019.01.132
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10.1016/j.ecoenv.2019.110062
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Unravelling mechanistic reasons for differences in performance of different Ti- and Bi-based magnetic photocatalysts in photocatalytic degradation of PPCPs.
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TiO2/graphene-based nanocomposites for water treatment: A brief overview of charge carrier transfer, antimicrobial and photocatalytic performance
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Tunable titanium metal–organic frameworks with infinite 1D Ti–O rods for efficient visible-light-driven photocatalytic H2 evolution
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10.1016/j.chemosphere.2019.01.084
Hierarchical biomimetic BiVO4 for the treatment of pharmaceutical wastewater in visible-light photocatalytic ozonation.
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A systematic review of the stability of finished pharmaceutical products and drug substances beyond their labeled expiry dates
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Enhanced dark adsorption and visible-light-driven photocatalytic properties of narrower-band-gap Cu2S decorated Cu2O nanocomposites for efficient removal of organic pollutants.
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Towards industrial implementation of Electro-Fenton and derived technologies for wastewater treatment: A review
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Simultaneous efficient adsorption and accelerated photocatalytic degradation of chlortetracycline hydrochloride over novel Fe-based MOGs under visible light irradiation assisted by hydrogen peroxide
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Bioinspired metal oxide particles as efficient wet air oxidation and photocatalytic oxidation catalysts for the degradation of acetaminophen in aqueous phase.
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10.1016/J.JCLEPRO.2018.10.183
Photocatalytic degradation of amoxicillin via TiO2 nanoparticle coupling with a novel submerged porous ceramic membrane reactor
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10.1016/J.JMRT.2019.07.017
Photocatalytic degradation of anti-inflammatory drug using POPD/Sb2O3 organic-inorganic nanohybrid under solar light
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Photocatalytic degradation of naproxen by a H2O2-modified titanate nanomaterial under visible light irradiation
Gongduan Fan (2019)
10.1016/J.SBSR.2019.100288
Electrochemical detection and photocatalytic performance of MoS2/TiO2 nanocomposite against pharmaceutical contaminant: Paracetamol
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10.1016/J.APSUSC.2019.05.299
Ultrasound-assisted heterogeneous degradation of tetracycline over flower-like rGO/CdWO4 hierarchical structures as robust solar-light-responsive photocatalysts: Optimization, kinetics, and mechanism
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Facile synthesis of g-C3N4/CdWO4 with excellent photocatalytic performance for the degradation of Minocycline
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10.1016/J.SSI.2018.12.016
Sonochemical synthesis of novel ZnFe2O4/CeO2 heterojunction with highly enhanced visible light photocatalytic activity
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Pharmaceuticals, illicit drugs and their metabolites in fish from Argentina: Implications for protected areas influenced by urbanization.
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Microemulsion based synthesis of promoted Fe–Co/MgO nanocatalyst: Influence of calcination atmosphere on the physicochemical properties, activity and light olefins selectivity for hydrogenation of carbon monoxide
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La2MnTiO6 double perovskite nanostructures as highly efficient visible light photocatalysts
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10.1016/j.jphotochem.2020.112463
Synthesis of CuWO4/Bi2S3 Z-scheme heterojunction with enhanced cephalexin photodegradation
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Double-shelled ZnSnO3 hollow cubes for efficient photocatalytic degradation of antibiotic wastewater
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10.1016/j.seppur.2019.116098
Solvothermal synthesis of a peony flower-like dual Z-scheme PANI/BiOBr/ZnFe2O4 photocatalyst with excellent photocatalytic redox activity for organic pollutant under visible-light
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A self-assembled urchin-like TiO2@Ag–CuO with enhanced photocatalytic activity toward tetracycline hydrochloride degradation
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Thermodynamics of removing crotamiton and its transformation byproducts from water by a rotating advanced oxidation contactor with zeolite/TiO2 composite sheets
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Tetracycline removal from aqueous solution by visible-light-driven photocatalytic degradation with low cost red mud wastes
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10.1016/J.CEJ.2019.122269
Highly flexible, core-shell heterostructured, and visible-light-driven titania-based nanofibrous membranes for antibiotic removal and E. coil inactivation
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10.1016/j.cocis.2020.04.008
Stimuli-responsive microemulsions: State-of-the-art and future prospects
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10.1016/j.jclepro.2020.120055
Facile synthesis of Z-scheme composite of TiO2 nanorod/g-C3N4 nanosheet efficient for photocatalytic degradation of ciprofloxacin
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10.1016/j.jece.2020.104065
A novel synthesis of Co2ZrO5 and m-ZrO2 nanoparticles by sono-precipitation and hydrothermal methods and their application in UV/Visible-photocatalytic studies
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Photolytic and photocatalytic degradation of nitrofurantoin and its photohydrolytic products
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10.1016/j.apsusc.2019.144287
Perovskite LaNiO3/TiO2 step-scheme heterojunction with enhanced photocatalytic activity
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10.1016/j.jece.2020.103726
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Enhanced photocatalytic degradation of levofloxacin by Fe-doped BiOCl nanosheets under LED light irradiation
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10.1016/j.jre.2020.01.011
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10.1016/j.apcatb.2020.119298
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10.1016/j.jclepro.2020.120217
Economic evaluation of typical metal production process: A case study of vanadium oxide production in China
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10.1016/j.seppur.2020.117518
Investigation of visible-light-driven photocatalytic tetracycline degradation via carbon dots modified porous ZnSnO3 cubes: Mechanism and degradation pathway
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10.1016/j.seppur.2019.116138
Effective photocatalytic degradation of sulfamethazine by CNTs/LaVO4 in suspension and dip coating modes
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10.1016/j.apcatb.2020.118716
Smart pathways for the photocatalytic degradation of sulfamethoxazole drug using F-Pd co-doped TiO2 nanocomposites
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10.1016/j.chemosphere.2020.127759
Simultaneous photocatalytic degradation of ibuprofen and H2 evolution over Au/sheaf-like TiO2 mesocrystals.
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10.1016/j.jhazmat.2020.122366
Anionic polyacrylamide-assisted construction of thin 2D-2D WO3/g-C3N4 Step-scheme heterojunction for enhanced tetracycline degradation under visible light irradiation.
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10.1016/j.seppur.2020.116800
Efficient photocatalytic degradation of furosemide by a novel sonoprecipited ZnO over ion exchanged clinoptilolite nanorods
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10.1016/j.molliq.2020.113530
Hybrid 2D/3D g-C3N4/BiVO4 photocatalyst decorated with RGO for boosted photoelectrocatalytic hydrogen production from natural lake water and photocatalytic degradation of antibiotics
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10.1016/j.apsusc.2020.146344
Microwave-assisted synthesis of a TiO2-CuO heterojunction with enhanced photocatalytic activity against tetracycline
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10.1016/J.SEPPUR.2019.115959
Fabrication of dual Z-scheme MIL-53(Fe)/α-Bi2O3/g-C3N4 ternary composite with enhanced visible light photocatalytic performance
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Pt–TiO2–Nb2O5 heterojunction as effective photocatalyst for the degradation of diclofenac and ketoprofen
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10.1016/j.jcis.2020.02.065
TBAOH assisted synthesis of ultrathin BiOCl nanosheets with enhanced charge separation efficiency for superior photocatalytic activity in carbamazepine degradation.
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10.1016/j.colsurfa.2019.123994
Two layered Bi-based borate photocatalysts MBi2B2O7 (M = Ca, Sr) for photocatalytic degradation and oxygen activation
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10.1016/J.CEJ.2019.122520
Enhancement of the oxidative removal of diclofenac and of the TiO2 rate of photon absorption in dye-sensitized solar pilot scale CPC photocatalytic reactors
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Photo-Fenton reaction for the degradation of sulfamethoxazole using a multi-walled carbon nanotube-NiFe2O4 composite
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Volumetric buffering of manganese dioxide nanotubes by employing ‘as is’ graphene oxide: An approach towards stable metal oxide anode material in lithium-ion batteries
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Green ZnO nanorod material for dye degradation and detoxification of pharmaceutical wastes in water
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10.1016/j.scitotenv.2019.134643
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10.1016/j.jmrt.2019.12.086
HZSM-5 zeolite supported boron-doped TiO2 for photocatalytic degradation of ofloxacin
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10.1016/j.mssp.2019.104829
Effect of synthesis route on the structural and morphological properties of WO3 nanostructures
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10.1016/j.cej.2019.123599
The enhanced photocatalytic performance toward carbamazepine by nitrogen-doped carbon dots decorated on BiOBr/CeO2: Mechanism insight and degradation pathways
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10.1016/j.materresbull.2019.110647
Effect of Ce on piezo/photocatalytic effects of Ba0.9Ca0.1CexTi1-xO3 ceramics for dye/pharmaceutical waste water treatment
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10.1016/j.matpr.2019.12.418
Hydrothermal synthesis of WO3 nanoparticles: Characterization and sonocatalytic study
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10.1016/J.SEPPUR.2019.115917
Facile synthesis of Bi5O7Br/BiOBr 2D/3D heterojunction as efficient visible-light-driven photocatalyst for pharmaceutical organic degradation
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