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Antifouling Coatings Via Tethering Of Hyperbranched Polyglycerols On Biomimetic Anchors

Dicky Pranantyo, L. Xu, K. Neoh, E. Kang, S. Teo
Published 2016 · Chemistry

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Hyperbranched polyglycerols (HPG) bearing terminal thiol moieties (HPG-SH) were synthesized via anionic-ring-opening multibranching polymerization of glycidol from pentaerythritol and subsequent 1,1′-carbonyldiimidazole (CDI) coupling with cysteamine. Bioinspired (1) N-dopamine maleimide (DM), (2) tannic acid (TA), and (3) polydopamine (PDA) were employed to produce monolayer, multilayer, and polymeric anchors, respectively, on stainless-steel (SS) substrates. Postfunctionalization of the biomimetic anchor-modified SS surfaces was enacted by tethering of HPG-SH via Michael addition or thiol–ene “click” reaction to confer surface hydrophilicity. The thickness and grafting density of HPG coatings could be controlled by tuning the degree of thiolation. In comparison to the pristine SS surface, the HPG-modified surfaces exhibited substantially reduced initial adhesion and inhibition of the biofilm formation of Gram-negative Pseudomonas sp. and Gram-positive Staphylococcus epidermidis. Qualitative and quantita...
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