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Chromophoric Self-Assembled Multilayers. Organic Superlattice Approaches To Thin-Film Nonlinear Optical Materials

D. Li, M. Ratner, T. Marks, Chong Hua Zhang, J. Yang, G. Wong
Published 1990 · Chemistry

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Poled polymer and acentric Langmuir-Blodgett films represent promising approaches to high-efficiency second harmonic generation (SHG) materials. Nevertheless, net achievable nonlinear optical (NLO) chromophore alignments, number densities, and alignment temporal stabilities are significant issues in the former materials, as are scattering microdomains, structural stability, and structural regularity, in the latter. The authors communicate here an alternative approach to thin-film NLO materials utilizing the sequential construction of covalently self-assembled chromophore-containing multilayer structures.



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