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Bifunctional Covalent Organic Frameworks With Two Dimensional Organocatalytic Micropores

Digambar Balaji Shinde, Sharath Kandambeth, Pradip Pachfule, Raya Rahul Kumar, Rahul Banerjee

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We report the successful incorporation of bifunctional (acid/base) catalytic sites in the crystalline organocatalytic porous COF (2,3-DhaTph). Due to the presence of acidic (catachol) and basic (porphyrin) sites, 2,3-DhaTph shows significant selectivity, reusability, and excellent ability to perform the cascade reaction.