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A Zwitterionic Triphosphenium Compound As A Tunable Multifunctional Donor

Stephanie C. Kosnik, Charles L. B. Macdonald

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We present a zwitterionic triphosphenium molecule which features dicoordinate, tricoordinate and tetracoordinate phosphorus centers in addition to a cyclopentadienyl moiety. Crystallographic, computational, electrochemical and spectroscopic data illustrate and rationalize the reactivity of this molecule as a multifunctional ligand for both transition metals and main group acceptors and suggest how the donor properties may be tuned.